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Granrodeo Performs Bungō Stray Dogs Opening Theme Song

Tsukito Totsuka) as Atsushi Nakajima (Light, Wind and Dreams), who came to Yokohama after being driven out of a poor orphanage that was attacked by a man-eating tiger. On the verge of starvation, he meets Dazai and gets a job helping at the detective agency. Because he's never had friends or family and was labeled as "useless," he lacks self-confidence. The website does not list his ability.

No Longer Human, Shayo), a member of the Armed Detective Agency. He's a suicide enthusiast who searches for a place to die. However, he doesn't like pain, and would prefer a lovers' suicide with a beautiful woman. He's aimless and elusive and doesn't bother anyone. His last job is said to be one of the "seven wonders of detective agencies." His ability is called "human elimination."

Aldnoah.Zero's Slaine Troyard) as Ryūnosuke Akutagawa (Rashōmon, Jigoku hen), a member of the notorious "Port Mafia" that operates by the harbor. With his black cloak and cold expression, he looks like the grim reaper when he walks the streets. His ability is called "Rashōmon."

Haikyu!!'s Asahi Azumane) as Doppo Kunikida (River Mist and Other Stories), a member of the Armed Detective Agency. He carries a notepad with the word "Ideal" written on the cover, and what is written inside are guides for life. He has a straight-laced personality and hates nothing more than schedules going awry. As a partner to the free-spirited Dazai, his troubles never end.

Hiroshi Kamiya (Attack on Titan's as Levi) as Rampo Edogawa (Private Detective Kogoro Akechi series), the great detective of the Armed Detective Agency. He possesses sharp observation skills that are acknowledged by his coworkers, and he settles difficult cases at the request of the police. Because of his self-confidence, his speech is brazen and child-like. His motto is "If you'll have me, everything will be ok!"

Durarara!!'s Mikado Ryūgamine) as Junichirō Tanizaki (Naomi, The Makioka Sisters), a seemingly-flirtatious young man who wears a baggy shirt and uses a pin to hold back his hair.

Kaze no Matasaburo), a member of the Armed Detective Agency. Before he was scouted, he lived in a rural area without electricity. He knows no suspicion, and will be understanding and considerate no matter who he is talking to. He has a lot of friends who call him "Ken-chan."

Maruzen Building. He's an enthusiastic scientists who boasts that "death" is the "ultimate experiment."

Takekurabe), a beautiful and intelligent woman who wears pants. She belongs to a commando unit that answers to the leader of Port Mafia, and has authority over the military group "Black Lizard." She adores Akutagawa and calls him "senpai."

Monogatari), a docile young lady who dresses in a kimono, but also a member of Port Mafia. As she holds a killing ability, she was found by the organization and raised as an assassin.

Kishô Taniyama (Attack on Titan's Jean, GRANRODEO vocalist) as Chūya Nakahara (Poems of the Goat), a top-level Port Mafia member who detests Osamu Dasai. He's short but he's quick and uses powerful martial arts.